Preheat oven to 350 degrees. Grease and flour 2 9-inch or 3 7-inch round cake pans. Line bottoms with parchment paper (see link in post). Reserve.
In a large bowl, beat eggs for 2-3 minutes on medium speed until they turn a pale yellow. Add in sugar and beat until well combined. Add in mayonnaise, coffee, and vanilla and beat until mixture is well blended.
In a medium bowl whisk together flour, baking soda, baking powder, salt and cocoa powder. Add flour mixture in 4 additions, mixing well between additions. Stir in chocolate chunks.
Divide batter evenly between prepared pans or until pans are half full. Do not overfill. Bake at 350 for 25 - 30 minutes or until a cake tester comes out clean. Allow to cool in pans on wire racks for 30 minutes. Then remove from pans and allow to cool until just slightly warm. Wrap warm cakes in plastic wrap and place in freezer while you prepare the cream cheese toffee bit filling and the buttercream & caramel frosting.